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•high-spin complexes for 3d metals* •strong-field ligands •low-spin complexes for 3d metals* * due to effect #2, octahedral 3d metal complexes can be low spin or high spin, but 4d and 5d metal complexes are alwayslow spin. Increasing ∆o the value of δoalso depends systematically on the metal: 1. The three molecular geometries relevant to this module are: square planar, tetrahedral, and octahedral. Square planar is the geometry where the molecule looks like a square plane. The complex which has the icasi number of unpaired electrons or all electrons paired and hence the lowest (or no) resultant spin or magnetic moment is called low spin (or spin paired) or ls complex. It is formed with strong tickl ligands and the complexes have higher values of crystal field splitting energy (δ 0 ). Diagrams for d 4, d 5, d 6, and d 7 metal ions have a discontinuity in energies as the ligand field is varied. The discontinuity, shown with the vertical line, represents complexes changing from high-spin to low-spin complexes. At the line, the spin pairing energy is equal to the crystal field splitting energy. Spin state affects the properties of complexes. High-spin complexes have a greater number of unpaired electrons as compared to low spin complexes. Octahedral high-spin complexes are paramagnetic in nature due to the presence of unpaired electrons. On the other hand, octahedral low spin complexes can be paramagnetic or diamagnetic. For octahedral fe(iii) complexes 5(d ), we must account for the existence of both high- and low-spin complexes. The electronic configuration of 3the free fe + ion is: for a low-spin octahedral complex such as [fe(cn) 6]3 dr. Said el-kurdi 12 for a 3high-spin octahedral complex such as [fef 6] , the five
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Complexes which are d8 high-spin are usually octahedral (or tetrahedral) while low-spin d8 complexes are generally 16-electron square planar complexes. •high-spin complexes for 3d metals* •strong-field ligands •low-spin complexes for 3d metals* * due to effect #2, octahedral 3d metal complexes can be low spin or high spin, but 4d and 5d metal complexes are alwayslow spin. Increasing ∆o the value of δoalso depends systematically on the metal: 1. The three molecular geometries relevant to this module are: square planar, tetrahedral, and octahedral. Square planar is the geometry where the molecule looks like a square plane. The most common examples of square planar complexes have metals that are d 8. This site was written by chris p. , college of saint benedict / saint john's university (retired) with other authors as noted on individual pages. In a tetrahedral complex, δt δ t is relatively small even with strong-field ligands as there are fewer ligands to bond with. It is rare for the δt δ t of tetrahedral complexes to exceed the pairing energy. Usually, electrons will move up to the higher energy orbitals rather than pair. Because of this, most tetrahedral complexes are high spin. Octahedral complexes with between 4 and 7 d electrons can be either high-spin or low-spin depending on the size of δ when the ligand field splitting has an intermediate value such that the two states have similar energies, then the two states can coexist in measurable amounts at equilibrium
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